Abstract
Achromatic metalens have the potential to significantly reduce the size and complexity of broadband imaging systems. A large variety of achromatic metalens has been proposed and most of them have the fixed achromatic band that cannot be actively modified. However, band-tunable is an important function in practical applications such as fluorescence microscopic imaging and optical detection. Here, we propose a bilayer metalens that can switch achromatic bands by taking the advantage of the high refractive index contrast of Sb2S3 between amorphous and crystalline state. By switching the state of Sb2S3, the achromatic band can be reversibly switched between the red region of visible spectrum (650-830 nm) and the near-infrared spectrum (830-1100 nm). This band-tunable design indicates a novel (to our knowledge) method to solve the problem of achromatic focusing in an ultrabroad band. The metalens have an average focusing efficiency of over 35% and 55% in two bands while maintaining diffraction-limited performance. Moreover, through proper design, we can combine different functionalities in two bands such as combining achromatic focusing and diffractive focusing. The proposed metalens have numerous potential applications in tunable displaying, detecting devices and multifunctional devices.
© 2022 Optica Publishing Group under the terms of the Optica Open Access Publishing Agreement
1. Introduction
Optical dispersion is a key characteristic of optical materials, which also plays an important role in full-color imaging devices. Researchers seek to manipulate the dispersion, since the manipulation of dispersion means numerous potential applications where information can be multiplexed. Enhanced dispersion can be utilized to separate the electromagnetic wave of different wavelength in the field of spectrometry and tomography. Similarly, eliminating the dispersion is widely needed for achromatic imaging. To properly control the optical dispersion will always cost a lot either in design or experimental work.
Recently, metalens, a kind of artificial period arranged sub-wavelength nanostructure, have shown unprecedented abilities in tailoring amplitude and phase. Like the conventional refractive optical lenses, metalens also suffer from chromatic aberration [1]. Over the past few years, a large variety of achromatic metalens have been demonstrated [2–12]. Especially for the achromatic bandwidth, the improvement from discrete wavelength [13–17] to continuous band [18–21] greatly enriches the color information density of imaging. After that, researchers have tried to broaden the achromatic bandwidth as much as possible. Broader bandwidth leads to the requirement of higher dispersion value difference. To satisfy the need for a large dispersion value difference, researchers have explored many approaches. A simple and effective way for dielectric metasurfaces is to increase the range of effective refractive index such as employing high refractive index materials and increasing the height of metaunit, but the resonance effect (nonlinearity of the phase curve) [22–25] may lead to low efficiency and focal length shift [26]. Reducing the NA of the metalens is another way but cannot fundamentally solve the problem. A feasible exploration direction is to increase the structural complexity or the freedom degree to obtain greater difference of dispersion values [27–29]. A group innovatively proposed a hybrid 3D architecture combining nanoholes with a phase plate [30], and another group proposed a fishnet-achromatic metalens [31]. By properly designing the shape and stereo structure, both groups proposed a metalens with an ultrabroad achromatic bandwidth over 650 nm in visible and near-infrared spectrum, which open up a new way to broaden the achromatic bandwidth.
Actually, changing the refractive index of the material can be equivalent to increasing the freedom degree [32–36]. To modulate the refractive index and achieve different functions, there are a lot of methods, such as combining metasurfaces with digital coding or phase change materials to provide dynamic reconfigurability. Phase change materials usually refer to materials whose optical properties experience significant change after phase transition, which is widely used in reconfigurable photonic devices. However, few researchers have paid attention to broaden the achromatic bandwidth with phase change material. If we apply the phase change material properly, not only can the operation band being broader, but it can also be modulated actively. For the latter, in previous studies, one structural design corresponds to only one operation band, which strongly hinders its application. Realizing band-tunable functionality means we can switch the achromatic band without any structural change which is of great significance for imaging system with multi band imaging requirements. For instance, combining general infrared thermal imager and visible camera, we can switch the operation band without any inconvenient replacement of optical instrument or extra cost of other optical instrument.
In this work, we proposed a bilayer dielectric metasurfaces that can achieve achromatic focusing in a broad continuous bandwidth from 650 nm to 1100 nm under the incidence of circularly polarized light. The achromatic region consists of two bands, including Band A (650-830 nm) and Band B (830-1100 nm). By changing the state of Sb2S3 metaunits, the achromatic band can be switched between Band A and Band B without any structural change. This design method can be used to solve the problem that achromatic focusing in an ultrabroad band by splitting one band into two which avoids the inherent disadvantage of a single large band. What’s more, the average efficiencies of Band A and Band B are over 35% and 55% respectively with a peak efficiency of 70% at wavelength 1000 nm, and the average focal shift percentages are both below 3%. In addition, these two bands can be designed differently including the focal length and dispersion state within a certain range owing to the bilayer structure which successfully separates the requirements of dispersion value and focusing phase. Due to its flexible manipulation ability, it has great potential in dual-functional devices such as combining achromatic metalens with diffractive metalens. Our design propose a method to broaden the achromatic bandwidth while keeping a high image quality. The tunable bandwidth for achromatic metalens is a novel function for multifunctional metasurfaces, which is of great significance to the broadband applications of meta-devices.
2. Principle and design
Figure 1 depicts the working schematic of the metalens. The achromatic band of metalens can be switched reversibly based on phase change material Sb2S3. For amorphous Sb2S3, it can satisfy the required dispersion values in Band A (650-830 nm). By applying pulse voltage to indium tin oxide (ITO) layer to heat up Sb2S3 to the crystalline state, it can satisfy the required dispersion values in Band B (830-1100 nm).
To achieve achromatic focusing in a broad bandwidth, each metaunit must be designed to satisfy the phase requirement at all design wavelengths. Assuming that the metalens deflect light by a position($r$) dependent angle($\theta $), then according to the generalized Snell’s law [37], we can give this relation [31]:
As a proof-of-concept, we design and simulate an achromatic metalens with focal length ${f_A} = 14{\mu}m$ in Band A and focal length ${f_B} = 11{\mu}m$ in Band B. To improve the manipulation ability of focusing phase, the bilayer structure is proposed to improve the degree of phase regulation which separates the requirements of focusing phase and dispersion values. This design aims to allow the metalens to simultaneously satisfy the dispersion and focusing phase distribution at the reference wavelength. Figure 2 shows the schematic diagram of a metaunit. In this configuration, the bottom layer composed of Sb2S3 annular pillars surrounded by silica. Here, the dimension value of Sb2S3 annular pillars $({R1,R2} )$ were adjusted to achieve the required dispersion values. The upper layer composed of rectangular Si metaunit with a fixed dimension ($L = 295\; nm$, $W = 120\; nm$) produces a phase (based on the Pancharatnam-Berry phase) by rotating different angles ($\alpha $) for all frequency light. A thin layer of ITO is placed between the SiO2 substrate and Sb2S3 metaunits to heat up and realize the phase transition of Sb2S3. By properly selecting the $\textrm{g}(\mathrm{\omega } )$ function, the upper layer metaunits with identical dispersion will not affect the required dispersion [21]. In other words, we can almost ignore the constant dispersion acting on the whole metasurfaces. It’s worth noting that the layer distance $\textrm{h} = 400\,\textrm{nm}$ is designed to be close to minimize the effect of wavefront divergence after the first layer, bur far enough to avoid layer coupling [17].
To realize the switching function, here phase change material Sb2S3 is used which is a new kind of ultralow loss non-volatile reversible phase change material. Its extinction coefficient k is close to zero from 650 nm to 1100 nm in both amorphous and crystalline states as shown in Fig. 3(b) [40]. By increasing the temperature higher than 573 K, the crystallization of Sb2S3 can be achieved and by heating Sb2S3 to its 801 K ${\pm} $ 18 K melting point and then rapidly quenching, the amorphization can be achieved [40]. And all these process can be realized by applying specific voltage pulse to ITO layer for a predefined time duration [40,41]. There is a contrast of refractive index of $\Delta n = 0.3 - 0.5$ between Band A and Band B which helps realize different dispersion values. Figure 3(c) shows simulated phase values for amorphous Sb2S3 element (black dotted curve) and crystalline Sb2S3 element (red dotted curve) in wavelength region 650-1100 nm. For a particular position and focal length of metalens, the required phase was plotted as linear functions (blue and green area). As is clearly shown in Fig. 3(c), the slope of the red dotted curve keep stable in Band B, but increase significantly in Band A. Similarly, the black dotted curve has a better fit than red one in Band A. Therefore, crystalline and amorphous Sb2S3 can meet the required value in Band B and Band A, respectively. The expanded phase formula in two bands can be written as follows:
To visualize the required phase and library, Fig. 4(c) plot the group delay for all simulated elements as red circles, with the group delay in Band B on the x-axis and with the group delay in Band A on the y-axis. In order to implement our designed metalens, we compared the group delay and $\Delta \varphi $ values for each library element (Eq. (8)) to those of the target values obtained from Eqs. (4) and (5) to select the best element for each lens position. The element selecting process can be regarded as minimizing an error function written as:
3. Result and discussion
Based on the above analysis, we design and simulate an achromatic metalens with ${f_A} = 14\; {\mu}m$ and ${f_B} = 11\; {\mu}m$, and the corresponding numerical aperture (NA) are 0.39 and 0.47, which are calculated by $NA = \sin [{\tan ^{ - 1}}(D/2f)]$. Under the illumination of right-handed circularly polarized plane wave, the FDTD Solutions (Lumerical Inc., Vancouver, BC, Canada) simulation result of a full metalens is performed in Fig. 5. To reduce the simulation time and ensure accuracy, the mesh grids of the metalens and propagation space are set as 30nm×30nm×30 nm and 40nm×40nm×40 nm respectively. The perfectly matched layer (PML) boundary condition is applied for the three axis. When Sb2S3 is in crystalline stage, metalens only work in Band B, as shown in Fig. 5(b). By applying a voltage pulses to ITO layer to realize the switch from crystalline stage to amorphous stage of Sb2S3, metalens can work in Band A, as shown in Fig. 5(a). From the axial intensity distributions, the most obvious finding is that the chromatic aberration is apparently reduced across the entire operation bandwidth, with the focal planes for all wavelengths lying very close to one another. For both two bands, the focal shifts percentage, defined as the percentage of actual focal length deviating from the ideal focal length, are below 3%. Actually, FDTD simulations for a full metalens will calculate the coupling effect between metalens elements. However, since the period of element $P = 0.35\; \mu m$ satisfy the Nyquist sampling law, writing as $p \le {\lambda / {2NA}}$, the coupling effect is almost negligible and it will not affect the design process. For an imaging system, diffraction limit of the focal spots plays an important role for imaging quality. The full widths at half-maximum (FWHM) are shown in Fig. 5(f), and they are all close to the diffraction limit, calculated by $\lambda /2NA$. In addition, the depth of focus (DOF) keep stable for each achromatic band and parasitic focal spots is almost eliminated. DOF can be obtained by calculating the FWHM of the intensity field at z-axis in the propagation plane [42]. It is apparent that the uneven DOF will lead to image blur so maintaining the stability of DOF in a large operation band is also a key point of high-quality imaging. All these features could be attributed to the comprehensive coverage of group delay space provided by the element library. Figure 5(e) shows the focusing efficiencies for two wavelength region.
For Band A and Band B, the simulated average focusing efficiency are higher than 35% and 55% respectively. The focusing efficiency is defined as below [43]:
Based on the manipulation ability of phase and dispersion, our design approach allows for one metasurfaces to exhibit different combinations of focal length and dispersion state as long as the required phase and dispersion values can be met. About the focal length, just like the example ${f_A} = {f_B} = 12\; {\mu}m$ discussed above, there is a numerical limiting relationship between ${f_A}$ and ${f_B}$. We outlined the distribution area of the group delay point map. Assuming that all the area can be met without considering the value of $\Delta \varphi $, we study how the required curve can lay down on this area. Actually, the designed focal length will significantly affect the maximum difference of required dispersion values. When the diameter of metalens D is $12\; {\mu}m$, the relationship of $N{A_A}$ and $N{A_B}$ is shown in Fig. 6(b). The value represented by the color is the coverage rate of the required dispersion. This figure implies that the value of $N{A_A}$ and $N{A_B}$ should not have great difference and both $N{A_A}$ and $N{A_B}$ should not be too large. In addition to the focal length, the dispersion state can also be adjusted. The dispersion state refers to achromatic focusing or diffractive focusing here. To realize this function, the required group delay in achromatic focusing band should meet a hyperbolic trend phase dispersion as before while the required group delay in the other band are all close to a fixed value. Here Band A and Band B correspond to diffractive focusing and achromatic focusing respectively. Unfortunately, the coverage area of group delay point map do not have enough span in the horizontal direction (in Band B). Therefore, we have to make a compromise in fulfilling the group delay by tilting the required line a bit as shown in Fig. 7(c).
The full lens simulation result using Lumerical FDTD is shown in Fig. 7(a) (b). The focal length shift in Band B is small enough for achromatic imaging while the focal length in Band A decrease with respect to wavelength. Under the $Fresnel$ approximation, the diffractive focal length of incident wavelength is:
As shown in Fig. 7(d), the theoretical focal length calculated by Eq. (10) fits well with the simulated focal length. By switching the state of Sb2S3, the function of metalens can be changed from achromatic imaging to tomography. The parasitic focal spots can be seen at wavelength $830\; nm$ in Band B, we attribute this to the sparse density of group delay point map at high group delays. Besides, the elements with higher group delay are always accompanied by low efficiency and poor phase match, which is unavoidable.
4. Conclusion
In conclusion, we have demonstrated a band-tunable achromatic metalens covering a bandwidth over 450 nm in near-infrared spectrum based on phase change material Sb2S3. By separating the requirement of dispersion value and focusing phase, the two layers metasurfaces composed of high efficiency and large difference of dispersion value elements have been designed. For both two bands, the average focusing efficiency is high enough for high quality imaging and the FWHM is near at diffraction limit. From another point of view, this design method proposed a new way to achieve broadband achromatic focusing by splitting one band into two. This design strategy can be readily extended to other spectrum by using other phase change material. Achieving the function of band-tunable for achromatic metalens is firstly proposed in infrared spectrum and this characteristic indicates the great potential in detecting, displaying and other multifunctional imaging applications.
Funding
National Natural Science Foundation of China (61774062, 61875057, 11674109, 11674107); Natural Science Foundation of Guangdong Province (2021A151501035); Science and Technology Program of Guangzhou (2019050001).
Disclosures
The authors declare no conflict of interest.
Data availability
Data underlying the results presented in this paper are not publicly available at this time but may be obtained from the authors upon reasonable request.
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