Abstract
Spatial hole burning prevents single-frequency operation of thin-disk lasers when the thin disk is used as a folding mirror. We present an evaluation of the saturation effects in the disk for disks acting as end mirrors and as folding mirrors, explaining one of the main obstacles toward single-frequency operation. It is shown that a twisted-mode scheme based on a multi-order quarter-wave plate combined with a polarizer provides an almost complete suppression of spatial hole burning and creates an additional wavelength selectivity that enforces efficient single-frequency operation.
© 2018 Optical Society of America under the terms of the OSA Open Access Publishing Agreement
1. INTRODUCTION
The various longitudinal modes of a laser cavity undergoing optical amplification in the same active medium experience the phenomenon of gain competition, which leads to the prevailing of one mode over all the others and thus to single-frequency operation [1]. A tiny difference of the effective gain seen by a mode is sufficient to initiate this prevailing process. However, the domination of one mode over all the others can be sustained only when the stimulated emission induced by this mode causes gain saturation not only for itself (self-saturation), but with equal strength also for the other modes (cross saturation). This cross saturation occurs when the amplification of the various modes addresses the same regions of the active medium, so that the amplification of one mode depletes also the population inversion experienced by the other modes. If the various modes address the distribution of the population inversion in different ways, as in the case of “spatial hole burning” (SHB) [1,2], the amplification process of one mode only partially affects the population inversion experienced by the other modes. Several modes can thus coexist in steady-state conditions in a linear laser cavity preventing single-frequency operation.
The principle of SHB and its relation to single-frequency operation is illustrated in Fig. 1. In the center of a linear cavity, the standing wave pattern of the 14th longitudinal mode (black continuous curves) has maxima where the 13th longitudinal mode (black dashed curves) has minima. Therefore, the depletion of the population inversion caused by the 14th mode reduces the gain of the 14th mode (self-saturation) but does not significantly decrease the gain of the 13th mode (negligible cross saturation). As a consequence, the gain competition between these two adjacent longitudinal modes is strongly suppressed, and the laser operates simultaneously in several longitudinal modes.
SHB is often eliminated by the use of unidirectional ring-laser cavities. However, this is not an option for high-power thin-disk lasers, as Faraday rotators, required to enforce the unidirectional operation, lack the power-handling capability [3]. A well-established method to eliminate SHB in a linear cavity is given by the so-called twisted-mode scheme [1,4–7] where the counter-propagating beams in the active medium have orthogonal polarizations so that no interference occurs. To our knowledge, this method has so far not been applied to thin-disk lasers, except in our previous work [8].
By reducing the length of a laser cavity (in the micrometer range for Yb:YAG as active medium), the effect of SHB in preventing single-frequency operation can be eliminated. Indeed for such a short cavity, only one longitudinal mode falls into the spectral region where the active medium has a gain. Yet, these short cavities are not apt for high-power lasers, as they cannot sustain modes with large transverse size. Wavelength selective elements as gratings or Fabry–Perot etalons could be used to favor one of the modes, but also in these cases, an efficient selectivity can be achieved only for relatively short cavity lengths.
Another method to suppress the disrupting effects of SHB and to achieve single-frequency operation is obtained by using a short active medium placed close to a cavity end mirror. This is often called a “gain-at-the-end” configuration. In fact, as can be deduced from Fig. 1, in this region, the intensity maxima of neighboring modes are located at similar positions so that these modes sample the active medium with nearly identical patterns. Thus, a strong cross saturation between neighboring modes exists, which leads to the prevailing of the dominant mode over the others. Because of this, a thin-disk laser with the disk acting as end-mirror M1 is suitable for high-power lasers in single-frequency operation given the mitigation of the effects of SHB and the power scalability of the thin disk [8–10].
Improper understanding of the “gain-at-the-end” configuration has sometimes led to erroneously neglecting SHB when the thin disk is used as a folding mirror of the resonator. In such a case, the SHB pattern is more complex than presented in Fig. 1 because it results from the interference of four circulating beams, as recognized by Vorholt and Wittrock in Ref. [11]. However, their model does not include the dependence on the distance between the active medium and the end mirror (see in Fig. 9). SHB for disks acting as folding mirrors has also been discussed for mode-locked lasers [12,13], though this is not applicable for continuous wave (cw) and ns pulses. This study aims to clarify the SHB effects taking place in thin-disk lasers and their relation to single-frequency operation.
In Section 2 we introduce the fundamentals of SHB for the simple situation presented in Fig. 1, similar to the studies in Refs. [14–16]. The obtained results are then applied in Section 3 to the case of thin-disk lasers with the thin disk acting as cavity end mirror. In this design, SHB favors longitudinal modes with a large frequency spacing from the lasing (saturating) mode, which can be easily suppressed using standard frequency selective elements. Section 4 presents SHB when the thin disk acts as a folding mirror. The resulting interference of four beams in the active medium increases the susceptibility for SHB. In Section 5, we apply the twisted-mode scheme [4–7] to this cavity layout to reduce the four-beam to a two-beam interference, nearly eliminating the SHB. It is concluded with Section 6 presenting an implementation of the twisted-mode scheme in a -switched thin-disk laser [17].
2. SPATIAL HOLE BURNING FOR A LINEAR CAVITY
In this section, the well-known principle of SHB is derived for the linear cavity in Fig. 2 by using the generic building block of an amplifier given in Fig. 3. In this amplifier, a saturating Gaussian beam at a wavelength passes an active medium and travels to a mirror M1, which is reflecting the beam back onto itself. Thus, the beam crosses the medium a second time. The origin of the coordinate system used to compute SHB is located in the center of the active medium with the propagation and , the transverse directions. The position- and time-dependent amplitude of the forward propagating beam inside the active medium ( with the length of the active medium ) can be written as
with the width of the transverse profile of the beam, the refractive index of the active medium, the time, the amplitude of the beam on its symmetry axis, and and the frequency and wavelength of the beam, respectively. For simplicity, we neglected the increase of amplitude occurring in the active medium. This simplification allows for analytical results and is well justified for low-gain media as the thin disk. Furthermore, it provides qualitatively valid results also for high-gain media. Note that the laser gain will be accounted for separately [see, e.g., Eq. (9)]. The corresponding backward propagating beam is given by where is the optical distance between the center of the active medium and M1 with the distance between the active medium and M1 (cf. Figs. 1 and 3). The total amplitude in the active medium resulting from the superposition of the two beams is thusThe position dependency of the time-averaged intensity distribution resulting from the two counter-propagating beams is given by
where is the intensity of a single laser beam on its symmetry axis. From this intensity distribution , it is possible to obtain the position-dependent density of the population inversion in the active material by using the known rate equation for a four-level laser [1]: where is the pump rate (homogeneous within the active medium), the saturation fluence, and the lifetime of the upper state. The decrease of the upper state population by the stimulated emission is proportional to the local intensity of the circulating light . The steady-state solution of this rate equation () readsIn Eq. (7), we assumed that , which is valid for a weakly saturating beam intensity, e.g., for a laser cavity with an out-coupling mirror of low reflectivity. (For efficient laser operation, high saturation of the active medium is required. In this case, this assumption does not hold. Nevertheless, the general behavior presented in this study remains valid).
The position-dependent gain is proportional to the local density of the population inversion and can be expressed as
where is the unsaturated gain.So far, we have described the SHB effect of the dominant laser beam with a wavelength amplified in a dual-pass configuration, as depicted in Fig. 3. As a next step, we evaluate the saturation spectrum of the active medium experienced by a second (probing) beam at a wavelength . This beam forms a similar interference pattern in the active medium slightly shifted relative to . The cross-saturation gain experienced by this beam is given by the integral
where is the incident laser power at wavelength . The gain can be described as the product of the unsaturated laser gain and the saturation spectrum , so that the output power isThe saturation spectrum for the dual-pass configuration of Fig. 3 is thus given by
Combining Eq. (8) with Eq. (11), we find
Inserting the time-averaged intensity of Eq. (4) into Eq. (12), and assuming that and are much larger than and , and also that , we find
To obtain this result, we have made use of the approximation
A plot of the saturation spectrum for realistic values of and is shown in Fig. 4 as a function of the wavelength of the probe beam assuming a saturating beam at . When applying these results to a cavity, it is necessary to take into account that the wavelengths and can have discrete values only as a consequence of the resonance conditions. For the simplified cavity layout in Fig. 2 with , the longitudinal modes neighboring the saturating mode are located exactly at the two maxima of , as indicated by the blue hollow circles in Fig. 4. These two modes experience thus a gain decrease due to saturation effects significantly smaller compared to the gain decrease at the saturating wavelength . Therefore, amplification of these neighboring modes occurs leading to disruption of single-frequency operation. Because the spectral distance between modes for realistic layouts of rod lasers with typical cavity round-trip length of about 0.1 m is 1.5 GHz (5 pm at 1030 nm), the suppression of the neighboring modes using selective elements would require extremely narrow spectral filters with active regulation to prevent significant cavity losses at the operating wavelength .
3. SPATIAL HOLE BURNING FOR A THIN DISK ACTING AS CAVITY END MIRROR
For a thin disk acting as a cavity end-mirror M1 (see Fig. 5), the effects related with SHB are mitigated. Indeed for this “gain-at-the-end” configuration, the intensity pattern in the active medium (see Fig. 6) changes so slowly with the wavelength that the maxima and minima of the intensity pattern of two neighboring axial cavity modes are located at similar positions (cf. Fig. 1). This implies that the cross saturation between neighboring modes is nearly identical to the self-saturation. In other words, the saturation spectrum is a slowly varying function of .
The reduction of gain caused by the saturation spectrum for thin-disk lasers with disks acting as cavity end mirrors can be quantified using Eq. (13) and setting (cf. Figs. 2 with 5):
is plotted in Fig. 7 as a function of the wavelength for a realistic thin-disk laser () having a saturating mode at . A long cavity was assumed in this case to provide an intra-cavity beam with large required for the high-power operation. Because of this, the wavelength difference between neighboring modes in the 1030 nm region is only about 0.25 pm (75 MHz) apart, as indicated by the vicinity of the blue hollow circles and the black hollow square in Fig. 7(b). Thus, competition between the various modes located around the broad minimum centered at 1030 nm exists, which can be used to achieve single-frequency operation. In Fig. 7(a), the red squares indicate the maxima of the saturation spectrum at a spectral distance of 2.11 nm (615 GHz) from . These modes could grow in the laser cavity and disrupt single-frequency operation. However, due to the large spectral distance of these maxima, the laser operation at these wavelengths can be easily suppressed by introducing a standard frequency selective element (e.g., a birefringent filter or a grating [18]) without active stabilization.4. SPATIAL HOLE BURNING FOR A THIN DISK AS A FOLDING MIRROR
A more stable output beam for variations of the thin-disk thermal lens can be obtained by using the thin disk as a folding mirror in a V-shaped cavity (see Fig. 8). The stability properties of a laser containing a thermal lens have been studied in [19]. The thermal lens splits the cavity into two parts. The part that is longer (effective length given by the B-element of the corresponding ABCD matrix) has a complex beam parameter that exhibits a linear (first-order) dependence on variations of the thermal lens. By contrast, the -parameter in the shorter part exhibits a second-order dependence on variations of the thermal lens around the center of stability. Thus, to minimize variations of size and divergence of the output beam, the out-coupling mirror has to be placed in the short part of the cavity. When the thin disk is used as an end mirror of the cavity, it would be necessary to use the rear side of the disk as an out-coupling mirror, which is not feasible. As a result, the beam out-coupled from a thin-disk laser with the disk acting as end mirror suffers from a large sensitivity to variations of the thermal lens of the active medium. On the contrary, in a V-shaped cavity, the disk is used as a folding mirror, and the out-coupling mirror can be placed in the short (stable) part of the cavity leading to an out-coupled beam insensitive to variations of the thermal lens [8].
In contrast to the simple linear cavity of Fig. 5, in the V-shaped cavity with the disk acting as folding-mirror M1, the consideration of the SHB requires the evaluation of the interference of four beams similar to what was presented in [11]. Following the same methodology of Section 2 to compute the interference pattern, we proceed first by omitting M2 and computing the interference of the four beams for the amplifier configuration shown in Fig. 9. In a second step, the other end mirror (M2) is considered: it provides the resonance condition for the cavity.
The amplitude of the first beam traveling within the active medium with refractive index from the disk front side toward the disk rear side can be described as
where is the propagation angle relative to the disk normal within the active medium. Again, we assume that the origin of the reference system is located at the center of the disk, thus at a distance from the disk’s rear and front sides. The second beam originates from the reflection on the high-reflection (HR) coating at the rear side of the disk (M1). Within the active medium, the amplitude of this second beam is given byA phase delay and an inversion of the propagation in direction has been used to obtain this second beam from the first one, while size and direction in and directions are unchanged. This beam travels to M3 (given in green in Fig. 9), which reflects the beam in itself (inversion of all three propagation directions) back toward the active medium. The amplitude of this back-reflected beam traveling in the active medium from the front side to the rear side takes the form
where is the optical distance between the active medium center and M3, with and as defined in Fig. 9.After a second reflection on the HR coating of the disk, a fourth beam moving from the disk rear side to the front side is ensued whose amplitude takes the form
The time-averaged intensity distribution resulting from the interference of the four traveling waves takes the form
when walk-off effects are neglected. This approximation is justified given the small thickness of the disk () relative to the typical size of the cavity eigenmodes () and the small angle ().An example of such an intensity pattern is shown in Fig. 10. By inserting Eq. (19) into Eqs. (8) and (11), the gain decrease related to the saturation effects is obtained:
The saturation spectrum for and is shown in Fig. 11(a) as a function of the probe beam wavelength . The self saturation is depicted by the black square. The gray shaded region in the spectral plot of represents rapid oscillations caused by the large optical distance between the active medium and the end-mirror M3. These rapid oscillations are visible in Fig. 11(b), where the horizontal axis is magnified by a factor of in the wavelength region around the saturating wavelength . In the corresponding cavity (), the modes (indicated by the blue empty circles) nearest the saturating mode experience the maximal values of . As the two neighboring modes (and others) have a larger small-signal gain, they will grow until they significantly contribute to the saturation of the gain medium. Hence, single-frequency operation is disrupted. Also in this case, a suppression of these modes would require an extremely narrow-band filter with active stabilization to prevent significant losses at the wavelength of the saturating mode.
5. TWISTED-MODE OPERATION OF A V-SHAPED THIN-DISK LASER
The twisted-mode scheme [4–7] represents a well-known possibility to eliminate SHB. Its principle is to insert two quarter-wave plates, one before and one after the active medium, as presented in Fig. 12(a), such that there is no interference in the active medium, because the two counter-propagating beams have orthogonal polarizations. The absence of the interference between the two circulating beams leads to the complete elimination of the SHB paving the way for single-frequency operation [20–23].
The twisted-mode scheme could be implemented also for thin-disk lasers with V-shaped cavities, as shown, e.g., in Fig. 12(b). Yet, contrary to the cavity of Fig. 12(a), in this case, the twisted-mode scheme does not completely eliminate the interference. The interference between the beams traveling to, and being back-reflected from, mirror M1 (rear side of the disk) cannot be eliminated. The resulting interference pattern, which is shown in Fig. 13, reduces thus from a four-beam to a two-beam interference, similar to Fig. 6.
This reduction of the four-beam interference to a two-beam interference can be seen in the mathematical expression of the saturation spectrum , which takes the form
similar to Eq. (14). This equation also represents the saturation spectrum for a unidirectional ring cavity, provided that is substituted by .Practically, this twisted-mode scheme can be implemented using only a single quarter-wave plate as shown in Fig. 12(b). This design is possible given the small incident angle that can be realized and the availability of commercial waveplates with retardation showing only small position and incident angle dependences (the retardation scales quadratically with the incident angle) [1,24,25].
The usage of a multi-order waveplate is advisable, as it provides a higher damage threshold compared to a single-order waveplate. Besides enabling the implementation of the twisted-mode scheme, the multi-order waveplate combined with a polarizer also acts as a birefringent filter [18,26]. The wavelength-dependent retardation in a round-trip that occurs in the four passes in the quarter-wave plate leads to a wavelength-dependent round-trip transmission :
where is the round-trip retardation experienced in the quarter-wave plate at the wavelength ( for four passes in a 1.5 mm thick quartz plate at 1030 nm). The logarithm is used to present the transmission as coefficient of the exponential in Eq. (10).The improved frequency selectivity achieved with the multi-order waveplate is demonstrated in Fig. 14. The black curve represents a schematic representation of the unsaturated round-trip gain of the cavity depicted in Fig. 12(b) using a thin disk made of Yb:YAG (). The red curve represents the round-trip gain when accounting for the saturation effects caused by the dominant mode at . It is computed by multiplying from Eq. (21) with the unsaturated gain (black curve). Because the modes located at the two maxima of this curve see a larger gain than the dominant laser mode, they will grow until their saturation effects become relevant. Single-frequency operation is thus disrupted. The blue curve is the total round-trip gain that also includes the wavelength-dependent transmission of Eq. (22) for a quarter-wave plate based on a 1.5 mm thick quartz plate. This curve shows maximal gain for . Hence, the twisted-mode scheme can also be used for V-shaped cavities to obtain single-frequency operation.
6. DEMONSTRATION OF A -SWITCHED THIN-DISK LASER OPERATED IN TWISTED MODE
For the measurement of the 2S-2P splitting in muonic helium ions [27,28], we realized a -switched thin-disk oscillator as sketched in Fig. 15(a). The disk was used as a folding mirror, and a multi-order quarter-wave plate was inserted in front of the disk to implement the twisted-mode scheme and to provide the additional polarization-dependent losses . The waveplate was acting also as a window for the pump module [see Fig. 15(b)], which shielded the hot front surface of the disk from air flows that would lead to optical distortions of the laser beam.
The other optical elements of the cavity, namely, the Pockels-cell (PC), a second quarter-wave plate, and a thin-film polarizer (TFP), were used to control the pre-lasing operation and the -switch dynamics as explained for a similar system in Ref. [8]. Pulses up to an energy of 110 mJ at a repetition rate of 800 Hz were delivered by the oscillator. This laser was operated flawlessly for several months at the high-intensity proton accelerator of the Paul Scherrer Institute, Villigen, Switzerland.
The effectiveness of the twisted-mode scheme in reducing SHB manifests itself also in the measured temporal profile of the emitted laser pulses. Without the quarter-wave plate, or with its axis misaligned, the SHB causes simultaneous lasing at a few longitudinal modes, resulting in mode beating with a frequency given by the round-trip time [8,30,31] [see Fig. 16(a)]. This beating (fast oscillations) is suppressed when the quarter-wave plate is correctly aligned, as demonstrated in Fig. 16(b). The measurement of the pulse trace is thus a sensitive method to show the suppression of multi-mode operation [30,31]. In principle, also a spectrometer could be used, but a resolution better than 50 MHz is needed.
7. CONCLUSIONS
In this paper, we presented the wavelength-dependent decrease of the gain in an active medium caused by saturation effects. This decrease has been expressed as for various linear-cavity layouts: simple cavity [Eq. (13) and Fig. 4], thin-disk laser with the thin disk acting as end mirror [Eq. (14) and Fig. 7], and thin-disk laser with the disk as folding mirror [Eq. (20) and Fig. 11]. We found that the spectral distance between adjacent minima and maxima in around the saturating wavelength is large when the disk is used as the end mirror of the cavity. By contrast, it is small when the disk is used as a folding mirror. Hence, the “gain-at-the-end” configuration allows for easy suppression of interference effects using standard selective elements as Fabry–Perot etalons. For the more elaborate geometry where the disk acts as a folding mirror, suppression of these maxima is more challenging, given the small spectral distance (in the order of 100 MHz).
We have demonstrated that the implementation of the twisted-mode scheme in thin-disk lasers with V-shaped layouts suppresses only partially the SHB in the disk. Using the twisted-mode scheme with a multi-order waveplate, an additional wavelength-dependent loss arises that is spectrally sufficiently narrow to suppress the residual SHB effects that prevent single-frequency operation. The simplicity, efficiency, and robustness (in term of optical damage) of this scheme pave the way for achieving single-frequency operation of thin-disk lasers in the multi-kW range.
Funding
Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung (SNF) (SNF 200021_165854); H2020 European Research Council (ERC) (ERC CoG. #725039, ERC StG. #279765); Eidgenössische Technische Hochschule Zürich (ETH) (ETH-35 14-1); ETH Femtosecond and Attosecond Science and Technology (ETH-FAST).
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